Supercooled Liquid Water and Ice Crystal Distributions Within Sierra Nevada Winter Storms

1983 ◽  
Vol 22 (11) ◽  
pp. 1875-1886 ◽  
Author(s):  
Mark F. Heggli ◽  
Larry Vardiman ◽  
Ronald E. Stewart ◽  
Arlen Huggins
Keyword(s):  
Sierra Nevada ◽  
Liquid Water ◽  
Supercooled Liquid ◽  
Ice Crystal ◽  
Winter Storms

scholarly journals Ice is born in low-mobility regions of supercooled liquid water

2019 ◽  
Vol 116 (6) ◽  
pp. 2009-2014 ◽  
Author(s):  
Martin Fitzner ◽  
Gabriele C. Sosso ◽  
Stephen J. Cox ◽  
Angelos Michaelides
Keyword(s):  
Liquid Water ◽  
Dynamical Behavior ◽  
Supercooled Liquid ◽  
Ice Nucleation ◽  
Water Molecules ◽  
Ice Crystal ◽  
Surrounding Water ◽  
Dynamical Heterogeneity ◽  
Complex Dynamical Behavior

When an ice crystal is born from liquid water, two key changes occur: (i) The molecules order and (ii) the mobility of the molecules drops as they adopt their lattice positions. Most research on ice nucleation (and crystallization in general) has focused on understanding the former with less attention paid to the latter. However, supercooled water exhibits fascinating and complex dynamical behavior, most notably dynamical heterogeneity (DH), a phenomenon where spatially separated domains of relatively mobile and immobile particles coexist. Strikingly, the microscopic connection between the DH of water and the nucleation of ice has yet to be unraveled directly at the molecular level. Here we tackle this issue via computer simulations which reveal that (i) ice nucleation occurs in low-mobility regions of the liquid, (ii) there is a dynamical incubation period in which the mobility of the molecules drops before any ice-like ordering, and (iii) ice-like clusters cause arrested dynamics in surrounding water molecules. With this we establish a clear connection between dynamics and nucleation. We anticipate that our findings will pave the way for the examination of the role of dynamical heterogeneities in heterogeneous and solution-based nucleation.

Mobile Microwave Radiometer Observations: Spatial Characteristics of Supercooled Cloud Water and Cloud Seeding Implications

1995 ◽  
Vol 34 (2) ◽  
pp. 432-446 ◽  
Author(s):  
Arlen W. Huggins
Keyword(s):  
Liquid Water ◽  
Microwave Radiometer ◽  
Particle Growth ◽  
Supercooled Liquid ◽  
Winter Storms ◽  
Stable Conditions ◽  
Research Aircraft ◽  
Orographic Clouds ◽  
Liquid Depth ◽  
Windward Slope

Abstract Previous studies of the spatial distribution of supercooled liquid water in winter storms over mountainous terrain were performed primarily with instrumented aircraft and to a lesser extent with scans from a stationary microwave radiometer. The present work describes a new technique of mobile radiometer operation that was successfully used during numerous winter storms that occurred over the Wasatch Plateau of central Utah to determine the integrated depth of cloud liquid water relative to horizontal position on the mountain barrier. The technique had the advantage of being able to measure total liquid from the terrain upward, without the usual terrain avoidance problems that research aircraft face in cloudy conditions. The radiometer also collected data during several storms in which a research aircraft could not be operated because of severe turbulence and icing conditions. Repeated radiometer transects of specific regions of the plateau showed significant variability in liquid water depth over 30–60-min time periods, but also revealed that the profile of orographically generated cloud liquid was consistent, regardless of the absolute quantities. Radiometer liquid depth generally increased across the windward slope of the plateau to a peak near the western edge of the plateau top and then decreased across the relatively flat top of the plateau. These observations were consistent with regions where maximum and minimum vertical velocities were expected, and with depiction of cloud liquid by accretional ice particle growth across the mountain barrier. A comparison of data from the mobile radiometer and a stationary radiometer verified the general decrease in liquid depth from the windward slope to the top of the plateau and also showed that many liquid water regions were transient mesoscale features that moved across the plateau. Implications of the results, relative to the seeding of orographic clouds, were that seeding aerosols released from valley-based generators could at times be inhibited by stable conditions from reaching appropriate super-cooled liquid water regions and, as found by others, the region of cloud most likely to be encountered by an AgI seeding agent released from the ground was also relatively warm compared to the ice-forming capability of the particular agent used in these experiments. Also, one convective case study that exhibited relatively warm temperatures in the cloud layer indicated that, even in conditions that permit vertical transport to supercooled liquid zones, sufficient time for ice particle growth and fallout from seeded plumes on this plateau may be lacking.

Aircraft Icing Measurements in East Coast Winter Storms

1995 ◽  
Vol 34 (1) ◽  
pp. 88-100 ◽  
Author(s):  
Stewart G. Cober ◽  
George A. Isaac ◽  
J. W. Strapp
Keyword(s):  
Liquid Water ◽  
East Coast ◽  
Supercooled Liquid ◽  
Aircraft Icing ◽  
Winter Storms ◽  
Horizontal Extent ◽  
Microphysical Parameters ◽  
Median Volume ◽  
East Coast Winter Storms ◽  
Water Contents

Abstract Analysis of the aircraft icing environments of East Coast winter storms have been made from 3 1 flights duringthe second Canadian Atlantic Storms Program. Microphysical parameters have been summarized and are compared to common icing intensity envelopes and to other icing datasets. Cloud regions with supercooled liquid water had an average horizontal extent of 4.3 km, with average droplet concentrations of 130 μ, liquid water contents of 0.13 g m-3, and droplet median volume diameters of 18 pm. In general, the icing intensity observed was classified as light, although moderate to severe icing was observed in several common synoptic situationsand several cases are discussed. Freezing drizzle was observed on four flights, and represented the most severeicing environment encountered.

The Mystery of Ice Crystal Multiplication in a Laboratory Experiment

2013 ◽  
Vol 71 (1) ◽  
pp. 89-97 ◽  
Author(s):  
Gianni Santachiara ◽  
Franco Belosi ◽  
Franco Prodi
Keyword(s):  
Laboratory Experiment ◽  
Supercooled Liquid ◽  
Ice Crystals ◽  
Formation Processes ◽  
Ice Crystal ◽  
Droplet Vaporization ◽  
Ice Nuclei ◽  
Cold Room ◽  
The Mean ◽  
Ice Multiplication

Abstract This paper addresses the problem of the large discrepancies between ice crystal concentrations in clouds and the number of ice nuclei in nearby clear air reported in published papers. Such discrepancies cannot always be explained, even by taking into account both primary and secondary ice formation processes. A laboratory experiment was performed in a cylindrical column placed in a cold room at atmospheric pressure and temperature in the −12° to −14°C range. Supercooled droplets were nucleated in the column, in the absence of aerosol ice nuclei, by injecting ice crystals generated outside in a small syringe. A rapid increase in the ice crystal concentration was observed in the absence of any known ice multiplication. The ratio between the mean number of ice crystals in the column, after complete droplet vaporization, and the number of ice crystals introduced in the column was about 10:1. The presence of small ice crystals (introduced at the top of the column) in the unstable system (supercooled droplets) appears to trigger the transformation in the whole supercooled liquid cloud. A possible explanation could be that the rapidly evaporating droplets cool sufficiently to determine a homogeneous nucleation.

scholarly journals A Three-Year Climatology of Cloud-Top Phase over the Southern Ocean and North Pacific

2011 ◽  
Vol 24 (9) ◽  
pp. 2405-2418 ◽  
Author(s):  
Anthony E. Morrison ◽  
Steven T. Siems ◽  
Michael J. Manton
Keyword(s):  
Southern Ocean ◽  
Liquid Water ◽  
North Pacific ◽  
North Pacific Ocean ◽  
Supercooled Liquid ◽  
Global Climate Models ◽  
Shortwave Radiation ◽  
Orthogonal Polarization ◽  
Temperature Range ◽  
Cloud Tops

Abstract Moderate Resolution Imaging Spectroradiometer (MODIS) Level 2 observations from the Terra satellite are used to create a 3-yr climatology of cloud-top phase over a section of the Southern Ocean (south of Australia) and the North Pacific Ocean. The intent is to highlight the extensive presence of supercooled liquid water over the Southern Ocean region, particularly during summer. The phase of such clouds directly affects the absorbed shortwave radiation, which has recently been found to be “poorly simulated in both state-of-the-art reanalysis and coupled global climate models” (Trenberth and Fasullo). The climatology finds that supercooled liquid water is present year-round in the low-altitude clouds across this section of the Southern Ocean. Further, the MODIS cloud phase algorithm identifies very few glaciated cloud tops at temperatures above −20°C, rather inferring a large portion of “uncertain” cloud tops. Between 50° and 60°S during the summer, the albedo effect is compounded by a seasonal reduction in high-level cirrus. This is in direct contrast to the Bering Sea and Gulf of Alaska. Here MODIS finds a higher likelihood of observing warm liquid water clouds during summer and a reduction in the relative frequency of cloud tops within the 0° to −20°C temperature range. As the MODIS cloud phase product has limited ability to confidently identify cloud-top phase between −5° and −25°C, future research should include observations from the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) and other space-based sensors to help with the classification within this temperature range. Further, multiregion in situ verification of any remotely sensed observations is vital to further understanding the cloud phase processes.

scholarly journals Seedability of Winter Orographic Clouds

1986 ◽  
Vol 43 ◽  
pp. 127-138 ◽  
Author(s):  
Geoffrey E. Hill
Keyword(s):  
Wind Speed ◽  
Liquid Water ◽  
Supercooled Liquid ◽  
Direct Measurements ◽  
Orographic Clouds ◽  
The Subject ◽  
Relationship Of ◽  
Increasing Precipitation ◽  
Cloud Top Temperature ◽  
Limiting Value

Abstract This article is a review of work on the subject of seedability of winter orographic clouds for increasing precipitation. Various aspects of seedability are examined in the review, including definitions, distribution of supercooled liquid water, related meteorological factors, relationship of supercooled liquid water to storm stage, factors governing seedability, and the use of seeding criteria. Of particular interest is the conclusion that seedability is greatest when supercooled liquid water concentrations are large and at the same time precipitation rates are small. Such a combination of conditions is favored if the cloud-top temperature is warmer than a limiting value and as the cross-barrier wind speed at mountaintop levels increases. It is also suggested that cloud seeding is best initiated in accordance with direct measurements of supercooled liquid water, precipitation, and cross-barrier wind speed. However, in forecasting these conditions or in continuation of seeding previously initiated, the cloud-top temperature and cross-barrier wind speed are the most useful quantities.

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